Glassy Nuclei in Amorphous Ice:Novel Evidence for the Two-Liquids Nature of Water(BestMasters)

无定型冰中的玻璃核:水的双液性质的新证据

化学史

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1032.5
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作      者
出  版 社
出版时间
2019年07月01日
装      帧
平装
ISBN
9783658263232
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页      码
76
语      种
英文
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图书简介
Christina Maria Tonauer finds novel evidence for the first-order nature of the transition between high-density amorphous ice (HDA) and low-density amorphous ice (LDA), supporting water’s liquid-liquid transition scenarios. Pressure-dependent crystallisation experiments of differently prepared expanded high-density amorphous ice samples (eHDA) and subsequent powder x-ray diffraction experiments disclose nucleation of LDA domains in bulk HDA, a typical feature of a first-order transition. The comparison of pressure-dependent crystallisation temperatures of eHDA samples with LDA nuclei and bulk LDA allows the estimation of the Laplace pressure and the size of a LDA nucleus.
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